Open Access
Subscription Access
Impact of Lockdown-Related Reduction in Anthropogenic Emissions on Aerosol Characteristics in the Megacity, Bengaluru
Continuous analytical measurements of the loading and optical properties of near-surface aerosols over the megacity Bengaluru, in south India, are examined for the impact of the national lockdown (LD) associated with COVID-19 pandemic. The near total shutdown of rail, road, and air traffic as well as total closure of most of the business establishments and IT industry, especially during the first phase of the LD, is found to dramatically reduce black carbon (BC) abundance. Within one week of the first week of the LD phase 1 (LD1), the ambient BC concentration at the urban centre came down to levels comparable to those reported for remote rural locations, primarily due to >60% reduction in BC from fossil fuel (BCff) emissions. On the other hand, BC from biomass burning (BCwb) did not show any conspicuous impact. Consequently, the fraction of BCwb to BC more than doubled and the spectral absorption coefficient increased from ~1.15 to ~1.4. The single scattering albedo increased from its prevailing mean value 0.66 before LD to 0.74 during LD1 and then gradually decreased to 0.68 with increasing relaxations on vehicular traffic. The results reveal the unequivocal role of vehicular emissions in impacting the aerosol loading and their optical properties over Bengaluru. The study also shows how the environment responded to the gradual relaxations in the subsequent phases of LD. It is interesting to note that a few spells of strong rainfall towards the fourth phase of the LD impacted the aerosols non-selectively leading to sharp decrease in all the quantities. However, owing to the non-selective nature of the washout this large reduction in loading did not impact the single scattering albedo, unlike the case with the LD.
Keywords
Black Carbon, COVID-19 Lockdown, Scattering Coefficients, Single Scattering Albedo.
User
Font Size
Information
- IPCC, Climate Change 2013: The Physical Science Basis. Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change (eds Stocker, T., Dahe, Q. and Plattner, G.-K.), Cambridge University Press, Cambridge, 2013.
- Jacobson, M. Z., Control of fossil-fuel particulate black carbon and organic matter, possibly the most effective method of slowing global warming. J. Geophys. Res., 2002, 107(D19), 4410; http://dx.doi.org/10.1029/2001JD001376.
- Ramanathan, V. and Carmichael, G., Global and regional climate changes due to black carbon. Nature, 2008, 221–227; http://dx. doi.org/10.1038/ngeo156.
- Babu, S. S. and Moorthy, K. K., Aerosol black carbon over a tropical coastal station in India. Geophys. Res. Lett., 2002, 29(23), 13-11–13-14; doi:10.1029/2002gl015662.
- Latha, K., Badrinath, K. V. S. and Moorthy, K. K., Impact of diesel vehicular emissions on ambient black carbon concentration at an urban location in India. Curr. Sci., 2004, 86(3), 451–453.
- Satheesh, S. K., Vinoj, V. and Moorthy, K. K., Weekly periodicities of aerosol properties observed at an urban location in India. Atmos. Res., 2011, 101(1–2), 307–313; doi:10.1016/j.atmosres. 2011.03.003.
- Hansen, A. D. A., Rosen, H. and Novakov, T., The aethalometer – an instrument for the real-time measurement of optical absorption by aerosol particles. Sci. Total Environ., 1984, 36, 191–196.
- Sandradewi, J., Prévôt, A. S. H., Weingartner, E., Schmidhauser, R., Gysel, M. and Altensperger, U., A study of wood burning and traffic aerosols in an Alpine valley using a multi-wavelength aethalometer. Atmos. Environ., 2008, 42, 101–112.
- Drinovec, L., Močnik, G., Zotter, P., Prévôt, A. S. H., Ruckstuhl, C., Coz, E. and Hansen, A. D. A., The ‘dual-spot’ Aethalometer: an improved measurement of aerosol black carbon with real-time loading compensation. Atmos. Meas. Tech., 2015, 8(5), 1965– 1979; doi:10.5194/amt-8-1965-2015.
- Weingartner, E., Saathoff, H., Schnaiter, M., Streit, N., Bitnar, B. and Baltensperger, U., Absorption of light by soot particles: determination of the absorption coefficient by means of aethalometers. J. Aerosol Sci., 2003, 34(10), 1445–1463; doi:10.1016/s00218502(03)00359-8.
- Kirchstetter, T. W., Novakov, T. and Hobbs, P. V., Evidence that the spectral dependence of light absorption by aerosols is affected by organic carbon. J. Geophys. Res.: Atmosphere, 2004, 109(D21); http://dx.doi.org/10.1029/2004JD004999.
- Kleidman, R., Martins, J. V., Townsend, H. K., Hall, J., Gibson, M. D. and Martin, R., New capability for in situ measurements of particulate matter using size-selecting nephelometers as part of the SPARTAN network. Paper presented at the AGU Fall Meeting Abstracts, 2018; https://ui.adsabs.harvard.edu/abs/2018AGUFM. A13I2558K
- Anderson, T. L. and Ogren, J. A., Determining aerosol radiative properties using the TSI 3563 integrating nephelometer. Aerosol Sci. Technol., 1998, 29(1), 57–69; doi:10.1080/02786829808965551.
- Jethva, H. T., Satheesh, S. K., Srinivasan, J. and Krishnamoorthy, K., How good is the assumption about visible surface reflectance in MODIS aerosol retrieval over land? A comparison with aircraft measurements over an urban site in India. IEEE Trans. Geosci. Rem. Sens., 2009, 47(7), 10.1109/TGRS.2008.2010221.
- Anand, N., Sunilkumar, K., Satheesh, S. K. and Krishna Moorthy, K., Entanglement of near-surface optical turbulence to atmospheric boundary layer dynamics and particulate concentration: implications for optical wireless communication systems. Appl. Opt., 2020, 59(5), 1471; doi:10.1364/ao.381737.
- Moosmüller, H., Chakrabarty, R. K., Ehlers, K. M. and Arnott, W. P., Absorption Ångström coefficient, brown carbon, and aerosols: basic concepts, bulk matter, and spherical particles. Atmos. Chem. Phys., 2011, 11(3), 1217–1225; doi:10.5194/acp-11-1217-2011.
- Sandradewi, J. et al., Using aerosol light absorption measurements for the quantitative determination of wood burning and traffic emission contributions to particulate matter. Environ. Sci. Technol., 2008, 42, 3316–3323; doi:10.1021/es702253m.
- Ångström, A., The parameters of atmospheric turbidity. Tellus, 1964, 16, 64–75.
- Stull, R. B., An Introduction to Boundary Layer Meteorology, Kluwer, Dordrecht, 1988, p. 666; http://dx.doi.org/10.1007/97894-009-3027-8
- Babu, S. S. and Moorthy, K. K., Anthropogenic impact on aerosol black carbon mass concentration at a tropical coastal station: a case study. Curr. Sci., 2001, 81(9), 1208–1214.
- Nair, V. S. et al., Wintertime aerosol characteristics over the IndoGangetic Plain (IGP): impacts of local boundary layer processes and long-range transport. J. Geophys. Res., 2007, 112, D13205; http://dx.doi.org/10.1029/2006 JD008099.
- Andrews, E. et al., Comparison of methods for deriving aerosol asymmetry parameter. J. Geophys. Res., 2006, 111, D05S04; doi:10.1029/2004JD005734
- Wiscombe, W. J. and Grams, G., The backscattered fraction in two-stream approximations. J. Atmos. Sci., 1976, 33, 2440e2451.
Abstract Views: 365
PDF Views: 139