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Transition Probability Approach for Direct Calculation of Coefficients of Configuration Interaction Wave Function


Affiliations
1 Division of Chemical Sciences, Indian Institute of Science Education and Research Kolkata, Mohanpur 741 246, India
 

To reduce the computation cost of configuration interaction (CI) method, a novel technique is used to calculate the coefficients of doubly excited determinants directly from orbital energies, orbital overlap matrix and electron population obtained from Hartree–Fock level run. This approach to approximate the coefficients of CI wave function is termed as transition probability approximated CI (TPA-CI). In principle, calculated dynamical electron correlation energies of TPA-CI and full CI (FCI) are equivalent. It is observed that computed TPA-CI correlation energies of hydrogen, water, ammonia and ozone are close to the FCI values, within 5% error. The potential energy curve of hydrogen molecule is also studied, and it is found that the energy is minimum at its equilibrium bond length.

Keywords

Configuration Interaction, Potential Energy Curve, Transition Probability Approximation, Wave Function.
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Abstract Views: 350

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  • Transition Probability Approach for Direct Calculation of Coefficients of Configuration Interaction Wave Function

Abstract Views: 350  |  PDF Views: 125

Authors

Arijit Bag
Division of Chemical Sciences, Indian Institute of Science Education and Research Kolkata, Mohanpur 741 246, India

Abstract


To reduce the computation cost of configuration interaction (CI) method, a novel technique is used to calculate the coefficients of doubly excited determinants directly from orbital energies, orbital overlap matrix and electron population obtained from Hartree–Fock level run. This approach to approximate the coefficients of CI wave function is termed as transition probability approximated CI (TPA-CI). In principle, calculated dynamical electron correlation energies of TPA-CI and full CI (FCI) are equivalent. It is observed that computed TPA-CI correlation energies of hydrogen, water, ammonia and ozone are close to the FCI values, within 5% error. The potential energy curve of hydrogen molecule is also studied, and it is found that the energy is minimum at its equilibrium bond length.

Keywords


Configuration Interaction, Potential Energy Curve, Transition Probability Approximation, Wave Function.

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DOI: https://doi.org/10.18520/cs%2Fv113%2Fi12%2F2325-2328